UKCCSRC Call 2 Project C2-214 . The dataset consists of six excel spreadsheets containing data from six dynamic operating scenarios for post-combustion CO2 capture on coal, implemented at the UKCCSRC’s PACT amine pilot facility. Critical plant parameters including flowrates, temperatures, pressure, solvent composition and CO2 capture rate are recorded. Additional steady-state baseload data and information regarding plant dimensions are provided in a separate word document. The dataset was generated as part of a pilot-scale test campaign which aimed to investigate the effect of differences in plant construction on response to dynamic operations, and to provide a proof-of-concept for the control of plant parameters using continuous, online solvent measurements. They may be of use to those interested in the dynamic modelling of post-combustion CO2 capture, for the purpose of model validation. A collaborative research paper with researchers from Imperial College London is planned.